Database : MEDLINE
Search on : Electrolytes [Words]
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[PMID]: 29511734
[Au] Autor:Zhao Q; Huang W; Luo Z; Liu L; Lu Y; Li Y; Li L; Hu J; Ma H; Chen J
[Ad] Address:State Key Laboratory of Elemento-Organic Chemistry and Key Laboratory of Advanced Energy Materials Chemistry, College of Chemistry, Nankai University, Tianjin 300071, China.
[Ti] Title:High-capacity aqueous zinc batteries using sustainable quinone electrodes.
[So] Source:Sci Adv;4(3):eaao1761, 2018 Mar.
[Is] ISSN:2375-2548
[Cp] Country of publication:United States
[La] Language:eng
[Ab] Abstract:Quinones, which are ubiquitous in nature, can act as sustainable and green electrode materials but face dissolution in organic electrolytes, resulting in fast fading of capacity and short cycle life. We report that quinone electrodes, especially calix[4]quinone (C4Q) in rechargeable metal zinc batteries coupled with a cation-selective membrane using an aqueous electrolyte, exhibit a high capacity of 335 mA h g with an energy efficiency of 93% at 20 mA g and a long life of 1000 cycles with a capacity retention of 87% at 500 mA g . The pouch zinc batteries with a respective depth of discharge of 89% (C4Q) and 49% (zinc anode) can deliver an energy density of 220 Wh kg by mass of both a C4Q cathode and a theoretical Zn anode. We also develop an electrostatic potential computing method to demonstrate that carbonyl groups are active centers of electrochemistry. Moreover, the structural evolution and dissolution behavior of active materials during discharge and charge processes are investigated by operando spectral techniques such as IR, Raman, and ultraviolet-visible spectroscopies. Our results show that batteries using quinone cathodes and metal anodes in aqueous electrolyte are reliable approaches for mass energy storage.
[Pt] Publication type:JOURNAL ARTICLE
[Em] Entry month:1803
[Cu] Class update date: 180311
[Lr] Last revision date:180311
[St] Status:In-Data-Review
[do] DOI:10.1126/sciadv.aao1761

  2 / 35713 MEDLINE  
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[PMID]: 29524329
[Au] Autor:Meran Z; Besinis A; De Peralta T; Handy RD
[Ad] Address:School of Biomedical and Biological Sciences, University of Plymouth, Drake Circus, Plymouth, PL4 8AA, UK.
[Ti] Title:Antifungal properties and biocompatibility of silver nanoparticle coatings on silicone maxillofacial prostheses in vitro.
[So] Source:J Biomed Mater Res B Appl Biomater;106(3):1038-1051, 2018 Apr.
[Is] ISSN:1552-4981
[Cp] Country of publication:United States
[La] Language:eng
[Ab] Abstract:Patients with facial prostheses suffer from yeast, Candida albicans, infections. This study aimed to determine the biocompatibility and antifungal properties of silicone facial prostheses coated with silver nanoparticles (Ag NPs) in vitro. Medical grade silicone discs were coated with 5 and 50 mg L dispersions of either Ag NPs or AgNO . Coatings were fully characterized using scanning electron microscopy and energy dispersive X-ray spectroscopy. The biocompatibility was examined using human dermal fibroblasts (Hs68), whereas antifungal efficacy was tested against C. albicans (NCPF-3179). The fibroblast viability was assessed by measuring lactate dehydrogenase (LDH) activity, protein content and tissue electrolytes. There were no effects on the LDH activity of fibroblast cell homogenates, and leak of LDH activity into external media remained low (0.1-0.2 IU mL ). Sublethal effects of Ag NP coatings on membrane permeability/ion balance was not observed, as measured by stable homogenate Na and K concentrations. Some Ag (13 mg L ) was detected from the AgNO coatings in the media, but total Ag remained below detection limit (<1.2 µg L ) for the Ag NP coatings; indicating the latter were stable. When fibroblasts grown on silver coatings were challenged with C. albicans, the Ag NP coating was effective at preventing fungal growth as measured by ethanol production by the yeast, and without damaging the fibroblasts. Ethanol production decreased from 43.2 ± 25.02 in controls to 3.6 µmol mL in all the silver treatments. Data shows that silicone prosthetic materials coated with Ag NPs are biocompatible with fibroblast cells in vitro and show antifungal properties. © 2017 Wiley Periodicals, Inc. J Biomed Mater Res Part B: Appl Biomater, 106B: 1038-1051, 2018.
[Pt] Publication type:JOURNAL ARTICLE
[Em] Entry month:1803
[Cu] Class update date: 180310
[Lr] Last revision date:180310
[St] Status:In-Data-Review
[do] DOI:10.1002/jbm.b.33917

  3 / 35713 MEDLINE  
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[PMID]: 29523536
[Au] Autor:Popoola VO; Lau BD; Tan E; Shaffer DL; Kraus PS; Farrow NE; Hobson DB; Aboagye JK; Streiff MB; Haut ER
[Ad] Address:Division of Acute Care Surgery, Department of Surgery, Johns Hopkins Hospital, Baltimore, MD.
[Ti] Title:Nonadministration of medication doses for venous thromboembolism prophylaxis in a cohort of hospitalized patients.
[So] Source:Am J Health Syst Pharm;75(6):392-397, 2018 Mar 15.
[Is] ISSN:1535-2900
[Cp] Country of publication:United States
[La] Language:eng
[Ab] Abstract:PURPOSE: Results of a study to characterize patterns of nonadministration of medication doses for venous thromboembolism (VTE) prevention among hospitalized patients are presented. METHODS: The electronic records of all patients admitted to 4 floors of a medical center during a 1-month period were examined to identify patients whose records indicated at least 1 nonadministered dose of medication for VTE prophylaxis. Proportions of nonadministered doses by medication type, intended route of administration, and VTE risk categorization were compared; reasons for nonadministration were evaluated. RESULTS: Overall, 12.7% of all medication doses prescribed to patients in the study cohort ( = 75) during the study period (857 of 6,758 doses in total) were not administered. Nonadministration of 1 or more doses of VTE prophylaxis medication was nearly twice as likely for subcutaneous anticoagulants than for all other medication types (231 of 1,112 doses [20.8%] versus 626 of 5,646 doses [11.2%], < 0.001). For all medications prescribed, the most common reason for nonadministration was patient refusal (559 of 857 doses [65.2%]); the refusal rate was higher for subcutaneous anticoagulants than for all other medication categories (82.7% versus 58.8%, < 0.001). Doses of antiretrovirals, immunosuppressives, antihypertensives, psychiatric medications, analgesics, and antiepileptics were less commonly missed than doses of electrolytes, vitamins, and gastrointestinal medications. CONCLUSION: Scheduled doses of subcutaneous anticoagulants for hospitalized patients were more likely to be missed than doses of all other medication types.
[Pt] Publication type:JOURNAL ARTICLE
[Em] Entry month:1803
[Cu] Class update date: 180310
[Lr] Last revision date:180310
[St] Status:In-Data-Review
[do] DOI:10.2146/ajhp161057

  4 / 35713 MEDLINE  
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[PMID]: 29522350
[Au] Autor:DuChene J; Tagliabue G; Welch AJ; Cheng WH; Atwater HA
[Ti] Title:Hot Hole Collection and Photoelectrochemical CO Reduction with Plasmonic Au/p-GaN Photocathodes.
[So] Source:Nano Lett;, 2018 Mar 09.
[Is] ISSN:1530-6992
[Cp] Country of publication:United States
[La] Language:eng
[Ab] Abstract:Harvesting non-equilibrium hot carriers from plasmonic-metal nanostructures offers unique opportunities for driving photochemical reactions at the nanoscale. While examples of hot electron-driven processes abound, the realization of plasmonic systems capable of harvesting hot holes from metal nanostructures has eluded the nascent field of plasmonic photocatalysis. Here, we fabricate gold/p-type gallium nitride (Au/p-GaN) Schottky junctions tailored for photoelectrochemical studies of plasmon-induced hot hole capture and conversion. Despite the presence of an interfacial Schottky barrier to hot hole injection of more than 1 eV across the Au/p-GaN heterojunction, plasmonic Au/p-GaN photocathodes exhibit photoelectrochemical properties consistent with the injection of hot holes from Au nanoparticles into p-GaN upon plasmon excitation. The photocurrent action spectrum of the plasmonic photocathodes faithfully follows the surface plasmon resonance absorption spectrum of the Au nanoparticles and open-circuit voltage studies demonstrate a sustained photovoltage during plasmon excitation. Comparison with Ohmic Au/p-NiO heterojunctions confirms that the vast majority of hot holes generated via interband transitions in Au are sufficiently hot to inject above the 1.1 eV interfacial Schottky barrier at the Au/p-GaN heterojunction. We further investigated plasmon-driven photoelectrochemical CO reduction with the plasmonic Au/p-GaN photocathodes, and observed improved selectivity for CO production over H evolution in aqueous electrolytes. Taken together, our results offer experimental validation of photoexcited hot holes more than 1 eV below the Au Fermi level and demonstrate a photoelectrochemical platform for harvesting hot carriers to drive solar-to-fuel energy conversion.
[Pt] Publication type:JOURNAL ARTICLE
[Em] Entry month:1803
[Cu] Class update date: 180309
[Lr] Last revision date:180309
[St] Status:Publisher
[do] DOI:10.1021/acs.nanolett.8b00241

  5 / 35713 MEDLINE  
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[PMID]: 29504748
[Au] Autor:Seifitokaldani A; Gabardo CM; Burdyny T; Dinh CT; Edwards JP; Kibria MG; Bushuyev OS; Kelley SO; Sinton D; Sargent EH
[Ad] Address:Department of Electrical and Computer Engineering , University of Toronto , 35 St. George Street , Toronto , Ontario M5S 1A4 , Canada.
[Ti] Title:Hydronium-Induced Switching between CO Electroreduction Pathways.
[So] Source:J Am Chem Soc;, 2018 Mar 09.
[Is] ISSN:1520-5126
[Cp] Country of publication:United States
[La] Language:eng
[Ab] Abstract:Over a broad range of operating conditions, many CO electroreduction catalysts can maintain selectivity toward certain reduction products, leading to materials and surfaces being categorized according to their products; here we ask, is product selectivity truly a property of the catalyst? Silver is among the best electrocatalysts for CO in aqueous electrolytes, where it reaches near-unity selectivity. We consider the hydrogenations of the oxygen and carbon atoms via the two proton-coupled-electron-transfer processes as chief determinants of product selectivity; and find using density functional theory (DFT) that the hydronium (H O ) intermediate plays a key role in the first oxygen hydrogenation step and lowers the activation energy barrier for CO formation. When this hydronium influence is removed, the activation energy barrier for oxygen hydrogenation increases significantly, and the barrier for carbon hydrogenation is reduced. These effects make the formate reaction pathway more favorable than CO. Experimentally, we then carry out CO reduction in highly concentrated potassium hydroxide (KOH), limiting the hydronium concentration in the aqueous electrolyte. The product selectivity of a silver catalyst switches from entirely CO under neutral conditions to over 50% formate in the alkaline environment. The simulated and experimentally observed selectivity shift provides new insights into the role of hydronium on CO electroreduction processes and the ability for electrolyte manipulation to directly influence transition state (TS) kinetics, altering favored CO reaction pathways. We argue that selectivity should be considered less of an intrinsic catalyst property, and rather a combined product of the catalyst and reaction environment.
[Pt] Publication type:JOURNAL ARTICLE
[Em] Entry month:1803
[Cu] Class update date: 180309
[Lr] Last revision date:180309
[St] Status:Publisher
[do] DOI:10.1021/jacs.7b13542

  6 / 35713 MEDLINE  
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[PMID]: 29521086
[Au] Autor:Berger FJ; Higgins TM; Rother M; Graf A; Zakharko Y; Allard S; Matthiesen M; Gotthardt JM; Scherf U; Zaumseil J
[Ti] Title:From Broadband to Electrochromic Notch Filters with Printed Monochiral Carbon Nanotubes.
[So] Source:ACS Appl Mater Interfaces;, 2018 Mar 09.
[Is] ISSN:1944-8252
[Cp] Country of publication:United States
[La] Language:eng
[Ab] Abstract:Dense layers of semiconducting single-walled carbon nanotubes (SWNTs) serve as electrochromic materials in the near-infrared with high optical density and high conductivity. Electrochromic cells with tunable notch filter properties instead of broadband absorption are created via highly selective dispersion of specific semiconducting SWNTs through polymer-wrapping followed by deposition of thick films by aerosol-jet printing. A simple planar geometry with spray-coated mixed SWNTs as the counter electrode renders transparent metal oxides redundant and facilitates complete bleaching within a few seconds through iongel electrolytes with high ionic conductivities. Monochiral (6,5) SWNT films as working electrodes exhibit a narrow absorption band at 997 nm (full width at half maximum of 55-73 nm) with voltage-dependent optical densities between 0.2 and 4.5 and a modulation depth of up to 43 dB. These (6,5) SWNT notch filters can retain more than 95 % of maximum bleaching for several hours under open circuit conditions. In addition, different levels of transmission can be set by applying constant low voltage (1.5 V) pulses with modulated width or by a given number of fixed short pulses.
[Pt] Publication type:JOURNAL ARTICLE
[Em] Entry month:1803
[Cu] Class update date: 180309
[Lr] Last revision date:180309
[St] Status:Publisher
[do] DOI:10.1021/acsami.8b00643

  7 / 35713 MEDLINE  
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[PMID]: 29520986
[Au] Autor:Capillo G; Silvestro S; Sanfilippo M; Fiorino E; Giangrosso G; Ferrantelli V; Vazzana I; Faggio C
[Ad] Address:Department of Chemical, Biological, Pharmaceutical and Environmental Sciences, University of Messina, Viale Ferdinando Stagno d'Alcontres, 31 98166, S.Agata-Messina, Italy.
[Ti] Title:Assessment of electrolytes and metals profile of the Faro Lake (Capo Peloro Lagoon, Sicily, Italy) and its impact on Mytilus galloprovincialis.
[So] Source:Chem Biodivers;, 2018 Mar 09.
[Is] ISSN:1612-1880
[Cp] Country of publication:Switzerland
[La] Language:eng
[Ab] Abstract:Faro Lake is a coastal meromictic lagoon with singular characteristics in the Mediterranean (Messina, Sicily - Italy). It is part of the Natural Oriented Reserve of Capo Peloro (38°15'57" N; 15° 37'50" E). In this area, traditional mollusc farming activity persists, producing "autochthonous" mussels. This study reports of the Mytilus galloprovincialis haemolymph chemical profile and water variables determination of one year-lasted survey (April 2016-March 2017). The determinations of electrolytes (Na+, Cl-, K+, Ca2+, Mg2+, P inorganic) and heavy metals in both Faro lake water and haemolymph have been carried out. Heavy metals are elements with high density and are quite toxic in low concentrations, such as Al, As, Co, Cr, Cu, Fe, Mg, Mn, Pb, Sn, Zn. Heavy metals toxicity depends, principally, on bioaccumulation processes. M. galloprovincialis is a good bio-indicator, ideal for assess levels of environmental pollution thanks to its biological, ecological and physiological characteristics. The results of this study showed a typical fluctuation range in haemolymph and water parameters, related to the water ones; chemical-physical parameters affected the ions (electrolytes and metals) levels in some period of the year. The study reports the interactions between biotic (Mytilus galloprovincialis) and abiotic (water parameters) components of Faro Lake, and creates reference data for further future study on the same area or on similar ones. This article is protected by copyright. All rights reserved.
[Pt] Publication type:JOURNAL ARTICLE
[Em] Entry month:1803
[Cu] Class update date: 180309
[Lr] Last revision date:180309
[St] Status:Publisher
[do] DOI:10.1002/cbdv.201800044

  8 / 35713 MEDLINE  
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[PMID]: 29519741
[Au] Autor:Kumar B; Strouse J; Swee M; Lenert P; Suneja M
[Ad] Address:Division of Immunology, Department of Internal Medicine, University of Iowa Hospitals and Clinics, 200 Hawkins Drive, Iowa City, IA 52242. Electronic address: Bharat-Kumar@UIowa.edu.
[Ti] Title:Hydralazine-associated vasculitis: Overlapping features of drug-induced lupus and vasculitis.
[So] Source:Semin Arthritis Rheum;, 2018 Jan 12.
[Is] ISSN:1532-866X
[Cp] Country of publication:United States
[La] Language:eng
[Ab] Abstract:INTRODUCTION: Hydralazine is an antihypertensive medication that has been associated with drug-induced lupus erythematosus (DIL) as well as ANCA-associated vasculitis (AAV). Although rare, early diagnosis is critical since drug cessation is the mainstay of therapy. This retrospective study aims to characterize the clinical, laboratory, and histopathologic features of this disease. METHODS: Once approval was obtained from the Institutional Review Board at the University of Iowa, all patients carrying a diagnosis of vasculitis (ICD9 code: 447.6 or ICD10 code: I77.6, I80, L95, M30, or M31) and positive ANCA lab results over the past 15 years were identified. Age, gender, comorbid conditions, medications taken over the prior 6 months, laboratory data, including electrolytes, urine studies and serologies, chest x-rays, CT scans, and pathologic biopsy records were abstracted from the electronic medical record. RESULTS: 323 cases of AAV were identified, of which 12 were exposed to hydralazine, all at the time of diagnosis. The average duration of hydralazine therapy was 22 months and mean cumulative dose was 146g. Patients were typically older (70.3 years old) with slight female preponderance (7 females). Eleven patients presented with dyspnea, fatigue, and unintentional weight loss. Five had polyarthralgias and 8 had lower extremity petechiae. All 12 patients were both ANA and ANCA positive. ANA titers ranged from 1:160 and 1:2560. Ten were of diffuse pattern while 2 were nucleolar. ANCA titers ranged from 1:320 to 1:2560. Eleven had a pANCA pattern while one had cANCA. All 12 patients were positive for histone and 11 were positive for myeloperoxidase antibodies. Eleven also had dsDNA antibodies, and 4 had anti-cardiolipin IgG or IgM antibodies. Nine patients were also hypocomplementemic (mean C3 level: 88.4mg/dL; mean C4 level: 16.5mg/dL). All patients had variable levels of proteinuria (1+ to 3+) and eleven had active urine sediment. Urine protein:creatinine ratios ranged from 0.2 to 1.7. Of the 6 patients who underwent kidney biopsy, all 6 showed pauci-immune crescentic glomerulonephritis. Seven patients had bilateral pulmonary interstitial infiltrates and four had pleural effusions on CT scan. Four had pericardial effusions as demonstrated by echocardiography. CONCLUSIONS: Hydralazine-associated vasculitis is a drug-associated autoimmune syndrome that presents with interstitial lung disease, hypocomplementemia, and pauci-immune glomerulonephritis. Patients have elements of both DIL and DIV, as manifested by high ANA and ANCA titers as well as the presence of histone and MPO antibodies. Further research is needed to understand the etiopathogenesis of this condition.
[Pt] Publication type:JOURNAL ARTICLE
[Em] Entry month:1803
[Cu] Class update date: 180309
[Lr] Last revision date:180309
[St] Status:Publisher

  9 / 35713 MEDLINE  
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[PMID]: 29499109
[Au] Autor:Shen BH; Armstrong BL; Doucet M; Heroux L; Browning JF; Agamalian M; Tenhaeff WE; Veith GM
[Ad] Address:Department of Chemical Engineering , University of Rochester , Rochester , New York 14627 , United States.
[Ti] Title:Shear Thickening Electrolyte Built from Sterically Stabilized Colloidal Particles.
[So] Source:ACS Appl Mater Interfaces;, 2018 Mar 08.
[Is] ISSN:1944-8252
[Cp] Country of publication:United States
[La] Language:eng
[Ab] Abstract:We present a method to prepare shear thickening electrolytes consisting of silica nanoparticles in conventional liquid electrolytes with limited flocculation. These electrolytes rapidly and reversibly stiffen to solidlike behaviors in the presence of external shear or high impact, which is promising for improved lithium ion battery safety, especially in electric vehicles. However, in initial chemistries the silica nanoparticles aggregate and/or sediment in solution over time. Here, we demonstrate steric stabilization of silica colloids in conventional liquid electrolyte via surface-tethered PMMA brushes, synthesized via surface-initiated atom transfer radical polymerization. The PMMA increases the magnitude of the shear thickening response, compared to the uncoated particles, from 0.311 to 2.25 Pa s. Ultrasmall-angle neutron scattering revealed a reduction in aggregation of PMMA-coated silica nanoparticles compared to bare silica nanoparticles in solution under shear and at rest, suggesting good stabilization. Conductivity tests of shear thickening electrolytes (30 wt % solids in electrolyte) at rest were performed with interdigitated electrodes positioned near the meniscus of electrolytes over the course of 24 h to track supernatant formation. Conductivity of electrolytes with bare silica increased from 10.1 to 11.6 mS cm over 24 h due to flocculation. In contrast, conductivity of electrolytes with PMMA-coated silica remained stable at 6.1 mS cm over the same time period, suggesting good colloid stability.
[Pt] Publication type:JOURNAL ARTICLE
[Em] Entry month:1803
[Cu] Class update date: 180308
[Lr] Last revision date:180308
[St] Status:Publisher
[do] DOI:10.1021/acsami.7b19441

  10 / 35713 MEDLINE  
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[PMID]: 29441917
[Ti] Title:Analysis of the necessity of serum electrolyte monitoring for up to eight weeks after the completion of anti-epidermal growth factor receptor antibody administration.
[So] Source:Pharmazie;71(7):402-407, 2016 Jul 07.
[Is] ISSN:0031-7144
[Cp] Country of publication:Germany
[La] Language:eng
[Ab] Abstract:Electrolyte disturbances are a known side effect of cetuximab (cmab) and panitumumab (pmab) administration and monitoring is recommended during and for at least 8 weeks after pmab administration. However, the recommended duration of electrolyte monitoring is not stated on the cmab package insert in the EU or Japan and no previous studies have investigated the appropriate monitoring period for cmab and pmab. We retrospectively investigated electrolyte levels in 16 cmab-treated patients and 7 pmab-treated patients between 1 June 2009 and 31 December 2014. The mean minimum levels of serum magnesium, potassium, and calcium were analyzed in these patients before administration (baseline) and in period A (during administration), period B (time of the last administration), period C (from the completion of administration to 4 weeks after), and period D (from 4-8 weeks after administration). Hypokalemia persisted until period D in 1 cmab-treated patient. Hypomagnesemia persisted until period D in two pmab-treated patients and hypokalemia persisted until period D in 1 pmab-treated patient. In addition, the serum magnesium levels in periods A, B, and C in the cmab-treated patients were significantly lower than the baseline level (P < 0.05). In pmabtreated patients, the serum magnesium levels in periods A, C, and D, and the serum calcium levels in periods A, B, and C were lower than the baseline levels (P < 0.05). These findings indicate that it is necessary to monitor electrolyte levels for at least 8 weeks after the completion of administration of cmab or pmab.
[Mh] MeSH terms primary: Antibodies, Monoclonal/adverse effects
Cetuximab/adverse effects
Electrolytes/blood
Receptor, Epidermal Growth Factor/antagonists & inhibitors
Water-Electrolyte Imbalance/chemically induced
[Mh] MeSH terms secundary: Adult
Aged
Antibodies, Monoclonal/therapeutic use
Antibodies, Monoclonal, Humanized/adverse effects
Antibodies, Monoclonal, Humanized/therapeutic use
Calcium/blood
Cetuximab/therapeutic use
Female
Humans
Hypokalemia/blood
Hypokalemia/chemically induced
Magnesium Deficiency/blood
Magnesium Deficiency/chemically induced
Male
Middle Aged
Monitoring, Physiologic
Retrospective Studies
Water-Electrolyte Imbalance/blood
[Pt] Publication type:JOURNAL ARTICLE
[Nm] Name of substance:0 (Antibodies, Monoclonal); 0 (Antibodies, Monoclonal, Humanized); 0 (Electrolytes); 6A901E312A (panitumumab); EC 2.7.10.1 (Receptor, Epidermal Growth Factor); PQX0D8J21J (Cetuximab); SY7Q814VUP (Calcium)
[Em] Entry month:1803
[Cu] Class update date: 180308
[Lr] Last revision date:180308
[Js] Journal subset:IM
[Da] Date of entry for processing:180215
[St] Status:MEDLINE
[do] DOI:10.1691/ph.2016.6537


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