Base de dados : MEDLINE
Pesquisa : D02.033.800.875.875 [Categoria DeCS]
Referências encontradas : 359 [refinar]
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[PMID]:28551204
[Au] Autor:Perales E; García JI; Pires E; Aldea L; Lomba L; Giner B
[Ad] Endereço:Facultad de Ciencias de la Salud, Universidad San Jorge, Autovía A-23 Zaragoza-Huesca Km. 299, Villanueva de Gállego, E-50830, Zaragoza, Spain.
[Ti] Título:Ecotoxicity and QSAR studies of glycerol ethers in Daphnia magna.
[So] Source:Chemosphere;183:277-285, 2017 Sep.
[Is] ISSN:1879-1298
[Cp] País de publicação:England
[La] Idioma:eng
[Ab] Resumo:Glycerol is currently considered a raw, renewable material, which can be used to synthesize new glycerol derivatives that may be used as green solvents. However, these compounds must be environmentally evaluated before their use. The acute ecotoxicity of a series of mono-, di-, and trialkyl ethers synthesized from glycerol for the crustacean Daphnia magna has been studied. The EC values of these ethers after 24 h of exposure were determined according to the OECD 202 protocol. Their possible structural-toxicity relationships according to different alkyl substituents have been discussed after applying different QSAR models (with the DARC-PELCO approach and topological parameters). The results of the immobilization test show that most of the glycerol derivatives studied exhibit relatively low ecotoxicity. There is a correlation between the lipophilicity and the increase of the toxic effect in the crustacean biomodel. Furthermore, the length and the number of the alkyl substituents and ecotoxicity are highly related.
[Mh] Termos MeSH primário: Daphnia/efeitos dos fármacos
Éteres de Glicerila/toxicidade
Relação Quantitativa Estrutura-Atividade
[Mh] Termos MeSH secundário: Animais
Ecossistema
Éteres de Glicerila/química
Interações Hidrofóbicas e Hidrofílicas
Modelos Biológicos
Poluentes Químicos da Água/toxicidade
[Pt] Tipo de publicação:JOURNAL ARTICLE
[Nm] Nome de substância:
0 (Glyceryl Ethers); 0 (Water Pollutants, Chemical)
[Em] Mês de entrada:1709
[Cu] Atualização por classe:170929
[Lr] Data última revisão:
170929
[Sb] Subgrupo de revista:IM
[Da] Data de entrada para processamento:170529
[St] Status:MEDLINE


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[PMID]:28376258
[Au] Autor:Ricciardi M; Passarini F; Vassura I; Proto A; Capacchione C; Cucciniello R; Cespi D
[Ad] Endereço:Department of Chemistry and Biology "Adolfo Zambelli", University of Salerno, Via Giovanni Paolo II 132, 84084, Fisciano (SA), Italy.
[Ti] Título:Glycidol, a Valuable Substrate for the Synthesis of Monoalkyl Glyceryl Ethers: A Simplified Life Cycle Approach.
[So] Source:ChemSusChem;10(10):2291-2300, 2017 May 22.
[Is] ISSN:1864-564X
[Cp] País de publicação:Germany
[La] Idioma:eng
[Ab] Resumo:The disposal of any waste by recovering it within the production plant represents the ultimate goal of every biorefinery. In this scenario, the selective preparation of monoalkyl glyceryl ethers (MAGEs) starting from glycidol, obtained as byproduct in the epichlorohydrin production plant, represents a very promising strategy. Here, we report the synthesis of MAGEs through the reaction of glycidol with alcohols catalyzed by a green homogeneous Lewis acids catalyst, such as Bi triflate, under very mild reaction conditions. To evaluate the green potential of the proposed alternative, a simplified life cycle assessment (LCA) approach was followed by comparing the environmental performance of the proposed innovative route to prepare MAGEs with that of the most investigated pathway from glycerol. A considerable reduction of all impact categories considered was observed in our experimental conditions, suggesting that the glycidol-to-MAGEs route can be a valuable integration to the glycerol-to-MAGEs chain. Thanks to the use of primary data within the LCA model, the results achieved are a very good approximation of the real case.
[Mh] Termos MeSH primário: Compostos de Epóxi/química
Éteres de Glicerila/síntese química
Propanóis/química
[Mh] Termos MeSH secundário: Catálise
[Pt] Tipo de publicação:JOURNAL ARTICLE
[Nm] Nome de substância:
0 (Epoxy Compounds); 0 (Glyceryl Ethers); 0 (Propanols); S54CF1DV9A (glycidol)
[Em] Mês de entrada:1707
[Cu] Atualização por classe:170705
[Lr] Data última revisão:
170705
[Sb] Subgrupo de revista:IM
[Da] Data de entrada para processamento:170405
[St] Status:MEDLINE
[do] DOI:10.1002/cssc.201700525


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[PMID]:28306545
[Au] Autor:Schulze T; Weldon PJ; Schulz S
[Ad] Endereço:.
[Ti] Título:Scent gland constituents of the Middle American burrowing python, Loxocemus bicolor (Serpentes: Loxocemidae).
[So] Source:Z Naturforsch C;72(7-8):265-275, 2017 Jul 14.
[Is] ISSN:0939-5075
[Cp] País de publicação:Germany
[La] Idioma:eng
[Ab] Resumo:Analysis by gas chromatography/mass spectrometry of the scent gland secretions of male and female Middle American burrowing pythons (Loxocemus bicolor) revealed the presence of over 300 components including cholesterol, fatty acids, glyceryl monoalkyl ethers, and alcohols. The fatty acids, over 100 of which were identified, constitute most of the compounds in the secretions and show the greatest structural diversity. They include saturated and unsaturated, unbranched and mono-, di-, and trimethyl-branched compounds ranging in carbon-chain length from 13 to 24. The glyceryl monoethers possess saturated or unsaturated, straight or methyl-branched alkyl chains ranging in carbon-chain length from 13 to 24. Alcohols, which have not previously been reported from the scent glands, possess straight, chiefly saturated carbon chains ranging in length from 13 to 24. Sex or individual differences in secretion composition were not observed. Compounds in the scent gland secretions of L. bicolor may deter offending arthropods, such as ants.
[Mh] Termos MeSH primário: Álcoois/análise
Boidae/metabolismo
Ácidos Graxos/análise
Éteres de Glicerila/análise
Lipídeos/análise
Glândulas Odoríferas/secreção
[Mh] Termos MeSH secundário: Animais
Feminino
Cromatografia Gasosa-Espectrometria de Massas
Masculino
Estados Unidos
[Pt] Tipo de publicação:JOURNAL ARTICLE
[Nm] Nome de substância:
0 (Alcohols); 0 (Fatty Acids); 0 (Glyceryl Ethers); 0 (Lipids)
[Em] Mês de entrada:1709
[Cu] Atualização por classe:170927
[Lr] Data última revisão:
170927
[Sb] Subgrupo de revista:IM
[Da] Data de entrada para processamento:170318
[St] Status:MEDLINE


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[PMID]:28214513
[Au] Autor:Huguet C; Fietz S; Rosell-Melé A; Daura X; Costenaro L
[Ad] Endereço:Departamento de Geociencias, Universidad de los Andes, A.A. 4976 Bogotá, Colombia.
[Ti] Título:Molecular dynamics simulation study of the effect of glycerol dialkyl glycerol tetraether hydroxylation on membrane thermostability.
[So] Source:Biochim Biophys Acta;1859(5):966-974, 2017 05.
[Is] ISSN:0006-3002
[Cp] País de publicação:Netherlands
[La] Idioma:eng
[Ab] Resumo:Archaeal tetraether membrane lipids span the whole membrane width and present two C isoprenoid chains bound by two glycerol groups (or one glycerol and calditol). These lipids confer stability and maintain the membrane fluidity in mesophile to extremophile environments, making them very attractive for biotechnological applications. The isoprenoid lipid composition in archaeal membranes varies with temperature, which has placed these lipids in the focus of paleo-climatological studies for over a decade. Non-hydroxylated isoprenoid archaeal lipids are typically used as paleo-thermometry proxies, but recently identified hydroxylated (OH) derivatives have also been proposed as temperature proxies. The relative abundance of hydroxylated lipids increases at lower temperatures, but the physiological function of the OH moiety remains unknown. Here we present molecular dynamics simulations of membranes formed by the acyclic glycerol-dialkyl-glycerol-tetraether caldarchaeol (GDGT-0), the most widespread archaeal core lipid, and its mono-hydroxylated variant (OH-GDGT-0) to better understand the physico-chemical properties conferred to the membrane by this additional moiety. The molecular dynamics simulations indicate that the additional OH group forms hydrogen bonds mainly with the sugar moieties of neighbouring lipids and with water molecules, effectively increasing the size of the polar headgroups. The hydroxylation also introduces local disorder that propagates along the entire alkyl chains, resulting in a slightly more fluid membrane. These changes would help to maintain trans-membrane transport in cold environments, explaining why the relative abundance of hydroxylated Archaea lipids increases at lower temperatures. The in silico approach aids to understand the underlying physiological mechanisms behind the hydroxylated lipid based paleo-thermometer recently proposed.
[Mh] Termos MeSH primário: Éteres de Glicerila/química
Bicamadas Lipídicas/química
Simulação de Dinâmica Molecular
[Mh] Termos MeSH secundário: Hidroxilação
Fluidez de Membrana
Modelos Moleculares
Temperatura Ambiente
[Pt] Tipo de publicação:JOURNAL ARTICLE; RESEARCH SUPPORT, NON-U.S. GOV'T
[Nm] Nome de substância:
0 (Glyceryl Ethers); 0 (Lipid Bilayers)
[Em] Mês de entrada:1708
[Cu] Atualização por classe:170831
[Lr] Data última revisão:
170831
[Sb] Subgrupo de revista:IM
[Da] Data de entrada para processamento:170220
[St] Status:MEDLINE


  5 / 359 MEDLINE  
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[PMID]:28117757
[Au] Autor:Bernal-Chávez SA; Pérez-Carreto LY; Nava-Arzaluz MG; Ganem-Rondero A
[Ad] Endereço:Division de Estudios de Posgrado (Tecnología Farmacéutica), Facultad de Estudios Superiores Cuautitlán, Universidad Nacional Autónoma de Mexico, Cuautitlán Izcalli 54740, Estado de Mexico, Mexico. q901108@hotmail.com.
[Ti] Título:Alkylglycerol Derivatives, a New Class of Skin Penetration Modulators.
[So] Source:Molecules;22(1), 2017 Jan 22.
[Is] ISSN:1420-3049
[Cp] País de publicação:Switzerland
[La] Idioma:eng
[Ab] Resumo:The absorption modulating activity of two alkylglycerol derivatives (batyl and chimyl alcohol) on skin barrier properties was evaluated. Biophysical tests such as transepidermal water loss (TEWL) and attenuated total reflectance-Fourier transform infrared (ATR-FTIR) spectroscopy, as well as in vitro skin permeation studies, were performed in order to determine the effect of these compounds as chemical absorption modulators. Four drugs were used as models: three NSAIDS (diclofenac, naproxen, and piroxicam) and glycyrrhizic acid. The results showed that treatment of the skin with alkylglycerols caused (i) a reduction on the amount of drug permeated; (ii) a reduction in TEWL; and (iii) changes in the ATR-FTIR peaks of stratum corneum lipids, indicative of a more ordered structure. All of these findings confirm that alkyl glycerols have an absorption retarding effect on the drugs tested. Such effects are expected to give rise to important applications in the pharmaceutical and cosmetic sectors, in cases where it is desirable for the drug to remain in the superficial layers of the skin to achieve a local effect.
[Mh] Termos MeSH primário: Portadores de Fármacos/farmacologia
Éteres de Glicerila/farmacologia
Permeabilidade/efeitos dos fármacos
Absorção Cutânea/efeitos dos fármacos
Pele/metabolismo
[Mh] Termos MeSH secundário: Administração Cutânea
Animais
Diclofenaco/administração & dosagem
Diclofenaco/metabolismo
Ácido Glicirrízico/administração & dosagem
Ácido Glicirrízico/metabolismo
Naproxeno/administração & dosagem
Naproxeno/metabolismo
Piroxicam/administração & dosagem
Piroxicam/metabolismo
Pele/efeitos dos fármacos
Espectroscopia de Infravermelho com Transformada de Fourier
Suínos
[Pt] Tipo de publicação:JOURNAL ARTICLE
[Nm] Nome de substância:
0 (Drug Carriers); 0 (Glyceryl Ethers); 13T4O6VMAM (Piroxicam); 144O8QL0L1 (Diclofenac); 39YR661C4U (batyl alcohol); 57Y76R9ATQ (Naproxen); 6FO62043WK (Glycyrrhizic Acid); UJ10V6YY6H (chimyl alcohol)
[Em] Mês de entrada:1705
[Cu] Atualização por classe:170523
[Lr] Data última revisão:
170523
[Sb] Subgrupo de revista:IM
[Da] Data de entrada para processamento:170125
[St] Status:MEDLINE


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[PMID]:28103528
[Au] Autor:Caimi AT; Parra F; de Farias MA; Portugal RV; Perez AP; Romero EL; Morilla MJ
[Ad] Endereço:Nanomedicine Research Program, Departamento de Ciencia y Tecnología, Universidad Nacional de Quilmes, Roque Saenz Peña 352, Bernal, B1876BXD, Argentina.
[Ti] Título:Topical vaccination with super-stable ready to use nanovesicles.
[So] Source:Colloids Surf B Biointerfaces;152:114-123, 2017 Apr 01.
[Is] ISSN:1873-4367
[Cp] País de publicação:Netherlands
[La] Idioma:eng
[Ab] Resumo:Ultradeformable archaeosomes (UDA) are nanovesicles made of total polar archaeolipids (TPA) from the archaea Halorubrum tebenquichense, soybean phosphatidylcholine and sodium cholate (3:3:1w/w). Fresh dispersions of UDA including different type of antigens are acknowledged as efficient topical vaccination agents. UDA dispersions however, if manufactured for pharmaceutical use, have to maintain colloidal stability upon liposomicidal processes such as sterilization and lyophilization ( UDA), needed to extend shelf life during storage. The remaining capacity of UDA to act as adjuvants was therefore tested here for the first time. Another unexplored issue addressed here, is the outcome of replacing classical antigen inclusion into nanovesicles by their physical mixture. Our results showed that UDA behaved as super-stable nanovesicles because of its high endurance during heat sterilization and storage for 5 months at 40°C. The archaeolipid content of UDA however, was insufficient to protect it against lyophilization, which demanded the addition of 2.5% v/v glycerol plus 0.07% w/v glucose. No significant differences were found between serum anti-ovalbumin (OVA) IgG titers induced by fresh or UDA upon topical application of 4 weekly doses at 600µg lipids/75µg OVA to Balb/c mice. Finally, UDA mixed with OVA elicited the same Th2 biased plus a non-specific cell mediated response than OVA encapsulated within UDA. Concluding, we showed that TPA is key component of super-stable nanovesicles that confers resistance to heat sterilization and to storage under cold-free conditions. The finding of UDA as ready-to-use topical adjuvant would lead to simpler manufacture processing and cheaper products. .
[Mh] Termos MeSH primário: Nanopartículas/química
Vacinação
[Mh] Termos MeSH secundário: Liofilização
Éteres de Glicerila/química
Esterilização
[Pt] Tipo de publicação:JOURNAL ARTICLE
[Nm] Nome de substância:
0 (Glyceryl Ethers); 0 (archaeol lipid)
[Em] Mês de entrada:1703
[Cu] Atualização por classe:170321
[Lr] Data última revisão:
170321
[Sb] Subgrupo de revista:IM
[Da] Data de entrada para processamento:170120
[St] Status:MEDLINE


  7 / 359 MEDLINE  
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[PMID]:27756152
[Au] Autor:Tang WZ; Yang ZZ; Sun F; Wang SP; Yang F; Lin HW
[Ad] Endereço:a Research Center for Marine Drugs, State Key Laboratory of Oncogenes and Related Genes, Department of Pharmacy , Renji Hospital, School of Medicine, Shanghai Jiao Tong University , Shanghai 200127 , China.
[Ti] Título:Leucanone A and naamine J, glycerol ether lipid and imidazole alkaloid from the marine sponge Leucandra sp.
[So] Source:J Asian Nat Prod Res;19(7):691-696, 2017 Jul.
[Is] ISSN:1477-2213
[Cp] País de publicação:England
[La] Idioma:eng
[Ab] Resumo:Chemical investigation on CH Cl extract of the marine sponge Leucandra sp. afforded two new compounds named leucanone A (1) and naamine J (2), together with eight known compounds (3-10). Their structures were elucidated on the basis of NMR spectroscopic analyses, and comparing with the literature. The cytotoxic activities of the compounds were evaluated against four cancer cell lines, and compound 2 showed mild cytotoxic activities against MCF-7, A549, HeLa, and PC9 cancer cell lines with IC values in the range of 20.1-45.3 µM.
[Mh] Termos MeSH primário: Alcaloides/isolamento & purificação
Antineoplásicos/isolamento & purificação
Imidazóis/isolamento & purificação
Lipídeos/isolamento & purificação
Poríferos/química
[Mh] Termos MeSH secundário: Alcaloides/química
Alcaloides/farmacologia
Animais
Antineoplásicos/química
Antineoplásicos/farmacologia
Ensaios de Seleção de Medicamentos Antitumorais
Éteres de Glicerila/química
Éteres de Glicerila/isolamento & purificação
Éteres de Glicerila/farmacologia
Células HeLa
Seres Humanos
Imidazóis/química
Imidazóis/farmacologia
Concentração Inibidora 50
Lipídeos/química
Lipídeos/farmacologia
Células MCF-7
Biologia Marinha
Estrutura Molecular
Ressonância Magnética Nuclear Biomolecular
[Pt] Tipo de publicação:JOURNAL ARTICLE
[Nm] Nome de substância:
0 (Alkaloids); 0 (Antineoplastic Agents); 0 (Glyceryl Ethers); 0 (Imidazoles); 0 (Lipids); 0 (leucanone A); 0 (naamine J)
[Em] Mês de entrada:1708
[Cu] Atualização por classe:170809
[Lr] Data última revisão:
170809
[Sb] Subgrupo de revista:IM
[Da] Data de entrada para processamento:161021
[St] Status:MEDLINE
[do] DOI:10.1080/10286020.2016.1240171


  8 / 359 MEDLINE  
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[PMID]:27880034
[Au] Autor:Cucciniello R; Ricciardi M; Vitiello R; Di Serio M; Proto A; Capacchione C
[Ad] Endereço:Department of Chemistry and Biology "Adolfo Zambelli", University of Salerno, Via Giovanni Paolo II, 132, 84084, Fisciano (SA), Italy.
[Ti] Título:Synthesis of Monoalkyl Glyceryl Ethers by Ring Opening of Glycidol with Alcohols in the Presence of Lewis Acids.
[So] Source:ChemSusChem;9(23):3272-3275, 2016 Dec 08.
[Is] ISSN:1864-564X
[Cp] País de publicação:Germany
[La] Idioma:eng
[Ab] Resumo:The present work deals with the production of monoalkyl glyceryl ethers (MAGEs) through a new reaction pathway based on the reaction of glycidol and alcohols catalyzed by Lewis acid-based catalysts. Glycidol is quantitatively converted with high selectivity (99 %) into MAGEs under very mild reaction conditions (80 °C and 0.01 mol % catalyst loading) in only 1 h using Al(OTf) or Bi(OTf) as catalyst. The proposed method enhances the choice of possible green synthetic approaches for the production of value-added products such as MAGEs.
[Mh] Termos MeSH primário: Álcoois/química
Compostos de Epóxi/química
Éteres de Glicerila/síntese química
Propanóis/química
[Mh] Termos MeSH secundário: Catálise
Química Verde
Ácidos de Lewis/química
[Pt] Tipo de publicação:JOURNAL ARTICLE
[Nm] Nome de substância:
0 (Alcohols); 0 (Epoxy Compounds); 0 (Glyceryl Ethers); 0 (Lewis Acids); 0 (Propanols); S54CF1DV9A (glycidol)
[Em] Mês de entrada:1706
[Cu] Atualização por classe:170607
[Lr] Data última revisão:
170607
[Sb] Subgrupo de revista:IM
[Da] Data de entrada para processamento:161124
[St] Status:MEDLINE
[do] DOI:10.1002/cssc.201600989


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[PMID]:27783695
[Au] Autor:Langsrud S; Steinhauer K; Lüthje S; Weber K; Goroncy-Bermes P; Holck AL
[Ad] Endereço:Nofima-Norwegian Institute of Food, Fisheries and Aquaculture Research, Osloveien 1, N-1430 Aas, Norway.
[Ti] Título:Ethylhexylglycerin Impairs Membrane Integrity and Enhances the Lethal Effect of Phenoxyethanol.
[So] Source:PLoS One;11(10):e0165228, 2016.
[Is] ISSN:1932-6203
[Cp] País de publicação:United States
[La] Idioma:eng
[Ab] Resumo:Preservatives are added to cosmetics to protect the consumers from infections and prevent product spoilage. The concentration of preservatives should be kept as low as possible and this can be achieved by adding potentiating agents. The aim of the study was to investigate the mechanisms behind potentiation of the bactericidal effect of a commonly used preservative, 2-phenoxyethanol (PE), by the potentiating agent ethylhexylglycerin (EHG). Sub-lethal concentrations of EHG (0.075%) and PE (0.675%) in combination led to rapid killing of E. coli (> 5 log reduction of cfu after 30 min), leakage of cellular constituents, disruption of the energy metabolism, morphological deformities of cells and condensation of DNA. Used alone, EHG disrupted the membrane integrity even at low concentrations. In conclusion, sub-lethal concentrations of EHG potentiate the effect of PE through damage of the cell membrane integrity. Thus, adding EHG to PE in a 1:9 ratio has a similar effect on membrane damage and bacterial viability as doubling the concentration of PE. This study provides insight about the mechanism of action of a strong potentiating agent, EHG, which is commonly used in cosmetics together with PE.
[Mh] Termos MeSH primário: Escherichia coli/efeitos dos fármacos
Etilenoglicóis/farmacologia
Éteres de Glicerila/farmacologia
Conservantes Farmacêuticos/farmacologia
[Mh] Termos MeSH secundário: Antibacterianos/farmacologia
Parede Celular/efeitos dos fármacos
Parede Celular/metabolismo
Cosméticos/química
Sinergismo Farmacológico
Metabolismo Energético
Microscopia Eletrônica de Transmissão
[Pt] Tipo de publicação:JOURNAL ARTICLE
[Nm] Nome de substância:
0 (Anti-Bacterial Agents); 0 (Cosmetics); 0 (Ethylene Glycols); 0 (Glyceryl Ethers); 0 (Preservatives, Pharmaceutical); 147D247K3P (ethylhexylglycerin); HIE492ZZ3T (phenoxyethanol)
[Em] Mês de entrada:1706
[Cu] Atualização por classe:170613
[Lr] Data última revisão:
170613
[Sb] Subgrupo de revista:IM
[Da] Data de entrada para processamento:161027
[St] Status:MEDLINE
[do] DOI:10.1371/journal.pone.0165228


  10 / 359 MEDLINE  
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[PMID]:26899807
[Au] Autor:Harries C; Mühlenbein S; Geier J; Pfützner W
[Ad] Endereço:Department of Dermatology and Allergology, Philipps University, D-35043 Marburg, Germany.
[Ti] Título:Allergic contact dermatitis caused by ethylhexylglycerin in both an ointment and a skin aerosol.
[So] Source:Contact Dermatitis;74(3):181-2, 2016 Mar.
[Is] ISSN:1600-0536
[Cp] País de publicação:England
[La] Idioma:eng
[Mh] Termos MeSH primário: Aerossóis/efeitos adversos
Dermatite Alérgica de Contato/etiologia
Éteres de Glicerila/efeitos adversos
Dermatoses da Mão/induzido quimicamente
Pomadas/efeitos adversos
[Mh] Termos MeSH secundário: Feminino
Seres Humanos
Meia-Idade
[Pt] Tipo de publicação:CASE REPORTS; JOURNAL ARTICLE
[Nm] Nome de substância:
0 (Aerosols); 0 (Glyceryl Ethers); 0 (Ointments); 147D247K3P (ethylhexylglycerin)
[Em] Mês de entrada:1612
[Cu] Atualização por classe:161230
[Lr] Data última revisão:
161230
[Sb] Subgrupo de revista:IM
[Da] Data de entrada para processamento:160223
[St] Status:MEDLINE
[do] DOI:10.1111/cod.12471



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